Bayly is a surname. Notable people with the surname include:
- Charles Bayly (fl. c. 1630–1680), the first overseas governor of the Hudson's Bay Company
- Christopher Alan Bayly (C.A. Bayly) (1945-2015), British historian specialising in British Imperial, Indian and global history
- Jaime Bayly (born 1965), Peruvian journalist and writer
- Joseph T. Bayly (1920–1986), American author and publishing executive
- Lewis Bayly (died 1631), an English author and Anglican bishop
- Sir Lewis Bayly (1857–1938), a British admiral
- Lorraine Bayly (born 1937), Australian actress
- Maurice Beddow Bayly (died 1962), English physician, anti-vivisection activist, and anti-vaccination campaigner
- Robert Bayly (born 1988), Irish footballer
- Thomas Bayly (Maryland politician) (1775–1829), Maryland congressman
- Thomas H. Bayly (1810–1856), Virginia congressman
- Thomas Haynes Bayly (1797–1839), English poet, songwriter and dramatist
- Thomas M. Bayly (1775–1834), Virginia congressman
- William Bayly (astronomer) (1737–1810), English astronomer
- William Bayly (barrister) (1540–1612), English barrister and politician
- William Alfred Bayly (1906–1934), New Zealand farmer and convicted murderer
- W. R. Bayly (1867–1937), educator in South Australia
- Zachary Bayly (military officer) (1841–1916), South African colonial military commander
- Zachary Bayly (planter) (1721–1769), planter and politician in Jamaica
See also
- The Bayly Baronets, a number of persons with the surname Bayly who held a baronetcy
- Bailey (surname)
- Bayley (disambiguation)
- Baillie (surname)
- Bailie (name)
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