Charles Bassett (1931–1966) was an American test pilot and astronaut.
Charles Bassett may also refer to:
- Charlie Bassett (1847–1896), American lawman and saloon keeper of the American Old West
- Charley Bassett (1863–1942), American baseball player
- Charles Bassett (basketball), American basketball coach
- Charles Philip Bassett, Canadian diplomat in the 1990s
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