Villarroel is a surname. Notable people with the surname include:
- Antoni de Villarroel (1656–1726), Spanish military commander, general commander of the Army of Catalonia in the War of the Spanish Succession
- Catherine Villarroel, fashion model and beauty queen from Bolivia
- Diego de Torres Villarroel (1693–1770), Spanish writer, poet, dramatist, doctor, mathematician, priest, professor of the University of Salamanca
- Gualberto Villarroel (1908–1946), head of state of Bolivia from December 20, 1943, to July 21, 1946
- Luis Villarroel (born 1981), Venezuelan diver
- Mario Enrique Villarroel Lander (born 1947), Venezuelan lawyer
- Moisés Villarroel (born 1976), Chilean football midfielder
- Néstor Guzmán Villarroel (born 1964), Bolivian politician and trade unionist
- Verónica Villarroel, Chilean soprano
See also
- Gualberto Villarroel Province, province in the La Paz Department, Bolivia
- Puerto Villarroel, locality in the Cochabamba Department in central Bolivia
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